We investigate the magnetic properties and the phonon-induced relaxation dynamics of the first regular Cr-9 antiferromagnetic (AF) ring, which represents a prototype frustrated AF ring. Geometrical frustration in Cr-9 yields an energy spectrum with twofold degenerate low-lying levels and a low-spin ground state. The electronic relaxation dynamics is probed by H-1-NMR through the temperature dependence of the spin-lattice relaxation rate 1/T-1. We develop a microscopic model that reproduces 1/T-1(T) curves, taking also into account the wipeout effect. By interpreting these measurements we determine the spin-phonon coupling strength and we investigate the decay of the cluster magnetization due to the spin-phonon interaction. We find that at very low temperatures, the relaxation is characterized by a single dominating Arrhenius-type relaxation process, whereas several relevant processes emerge at higher temperatures. In addition, we calculate the temperature andmagnetic field dependence of level lifetimes.
Relaxation dynamics in the frustrated Cr-9 antiferromagnetic ring probed by NMR / E. Garlatti, S. Bordignon, S. Carretta, G. Allodi, G. Amoretti, R. De Renzi, A. Lascialfari, Y. Furukawa, G.A. Timco, R. Woolfson, R.E.P. Winpenny, P. Santini. - In: PHYSICAL REVIEW. B. - ISSN 2469-9969. - 93:2(2016 Jan 29). [10.1103/PhysRevB.93.024424]
Relaxation dynamics in the frustrated Cr-9 antiferromagnetic ring probed by NMR
A. Lascialfari;
2016
Abstract
We investigate the magnetic properties and the phonon-induced relaxation dynamics of the first regular Cr-9 antiferromagnetic (AF) ring, which represents a prototype frustrated AF ring. Geometrical frustration in Cr-9 yields an energy spectrum with twofold degenerate low-lying levels and a low-spin ground state. The electronic relaxation dynamics is probed by H-1-NMR through the temperature dependence of the spin-lattice relaxation rate 1/T-1. We develop a microscopic model that reproduces 1/T-1(T) curves, taking also into account the wipeout effect. By interpreting these measurements we determine the spin-phonon coupling strength and we investigate the decay of the cluster magnetization due to the spin-phonon interaction. We find that at very low temperatures, the relaxation is characterized by a single dominating Arrhenius-type relaxation process, whereas several relevant processes emerge at higher temperatures. In addition, we calculate the temperature andmagnetic field dependence of level lifetimes.File | Dimensione | Formato | |
---|---|---|---|
199.pdf
accesso aperto
Tipologia:
Publisher's version/PDF
Dimensione
1.87 MB
Formato
Adobe PDF
|
1.87 MB | Adobe PDF | Visualizza/Apri |
Pubblicazioni consigliate
I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.